Factors affecting bioactivity (Beneficial or adverse effects of a drug on living matter.)

Redox potential - Tendency that a compound has to give or recieve electrons.

Eg. Riboflavin, ε0 = -0.185 V shows its effect on living matter whereas Dichlororiboflavin, ε0 = -0.095 V cannot be used as a drug.

Bioisosterism - Compounds or groups that posses similar physical properties.

Classical bioisosteres - Similarities of shape and electronic configuration of atoms with which they are replaced.

Univalent atoms/groups such as Cl, Br, I etc

Bivalent atoms/groups such as R-O-R, R-S-R etc

Trivalents atoms/groups such as -P=, -N=

Tetravalent atoms/groups such as =C=, =N= etc

Ring equivalent atoms/groups

Eg. Replacement of -NH2 in Carbutamide
to -CH3 in Tolbutamide

Non Classical bioisosteres - Functional group with dissimilar electronic configuration.

Halogen

Catechol

Ether

Carbonil group

Hydroxil group

Eg. Ring VS Noncyclic structure of Diethylstilbestrol and 17-beta oectradiol.

Lipophilicity - Affinity of a drug for a Lipid environment.

Its measured as Partition coefficient or Distribution coefficient.

It is the result of intermolecular forces present in a solute and the two phases it partitions

Eg. CYP450 metabolism - Metabolic rate increases with increased Lipophilicity.

Inductive effect - Ability to either donate or withdraw electron from adjacent atom or functional group.

Eg. Penicillin V is superior to Penicillin G because it has electron withdrawing effect that allows Penicillium V to have better bioavailability.

Resonance - A way of describing a molecule having delocalized set of electrons which cannot be expressed by a single structure.

Drug having resonance will have its bioactivity being reduced or increased by another functional group.

Eg. Penicillin V has better bioavailability than Penicillin G as the ether oxygen on Penicillin V can be electron donating via resonance which is absent in Penicillin G.

Solubility- Drug must be in solution form before it is absorbed in the body to produce biological activity.

Factors affecting solubility

Particle size - As size decreases, solubility increases

Boiling and melting point - As MP/BP increases, solubility decreases

Temperature - As temperature increases, solubility increases

pH, Nature of solvent, Pressure, Common ion effect etc

Methods to improve solubility

Structural modifications

Use of cosolvents (Ethanol, Sorbitol)

Employing surfactants

Complexations

Hydrogen bonding - dipole-dipole interaction between H atoms in a polar bond.

Intermolecular H bonding - occurs between two or more molecules of same or different compound.

Intramolecular H bonding - occurs between two atom of the same molecules.

Eg. 1-phenyl 2,3- dimethyl 5- pyrazolone has analgesic activity and 1-phenyl- 3- methyl-5- pyrazolone is inactive.

Spatial consideration - Any change in stereospecificity will affect its activity

Optical isomers - Physical properties of both the enantiomers are identical. Eg. (R)-(+)-Thalidomide is a sedative whereas (S)-(-)-Thalidomide is a teratogen.

Geometric isomers - Physical properties of
both the enantiomers are different. Eg.
Cisplatin is a effective anti-cancer drug

whereas Transplatin is not effective at all.

Ionisation and pH - Protonation or deprotonation resulting in charged molecules.

The rate of drug absorption is directly proportional to the conc of the drug at absorbable form.

Ionization form imparts good water solubility to the drug which is required to binding of drug and receptor interaction.

Unionised form helps the drug to cross the cell membrane.

Eg. Phenytoin injection must be adjusted to pH 12 with sodium hydroxide to obtain 99.8% of the drug in ionised form.

Partition coefficient - Equilibrium constant of drug concentration for unionised molecule in two phases.

Affected by factors such as

pH

Cosolvents

Surfactants

Complexation

Eg. Phenobarbitone has a high lipid/water Partition coefficient whereas Thiopentone sodium has value about 100 and it is highly lipid soluble therefore used as ultra-short acting barbiturates.